/* ---------------------------------------------------------------------- LAMMPS - Large-scale Atomic/Molecular Massively Parallel Simulator http://lammps.sandia.gov, Sandia National Laboratories Steve Plimpton, sjplimp@sandia.gov Copyright (2003) Sandia Corporation. Under the terms of Contract DE-AC04-94AL85000 with Sandia Corporation, the U.S. Government retains certain rights in this software. This software is distributed under the GNU General Public License. See the README file in the top-level LAMMPS directory. ------------------------------------------------------------------------- */ /* ---------------------------------------------------------------------- Contributing authors: Kristen Fichthorn, Tonnam Balankura, Ya Zhou (Penn State University) ------------------------------------------------------------------------- */ #include <cmath> #include <cstdio> #include <cstdlib> #include "pair_momb.h" #include "atom.h" #include "comm.h" #include "force.h" #include "neigh_list.h" #include "memory.h" #include "error.h" #include "citeme.h" using namespace LAMMPS_NS; static const char cite_momb[] = "Pair style momb:\n\n" "@Article{pair_momb_2015,\n" "title = {A force field for describing the polyvinylpyrrolidone-mediated" " solution-phase synthesis of shape-selective Ag nanoparticles.},\n" "volume = {118},\n" "number = {6},\n" "url = {http://dx.doi.org/10.1021/jp412098n},\n" "doi = {10.1021/jp412098n},\n" "journal = {J. Phys. Chem. C},\n" "author = {Zhou, Ya, Wissam A. Saidi, and Kristen A. Fichthorn},\n" "year = {2014},\n" "pages = {3366--3374}\n" "}\n\n"; /* ---------------------------------------------------------------------- */ PairMomb::PairMomb(LAMMPS *lmp) : Pair(lmp) { if (lmp->citeme) lmp->citeme->add(cite_momb); } /* ---------------------------------------------------------------------- */ PairMomb::~PairMomb() { if (allocated) { memory->destroy(setflag); memory->destroy(cutsq); memory->destroy(cut); memory->destroy(d0); memory->destroy(alpha); memory->destroy(r0); memory->destroy(c); memory->destroy(rr); memory->destroy(morse1); memory->destroy(offset); } } /* ---------------------------------------------------------------------- */ void PairMomb::compute(int eflag, int vflag) { int i,j,ii,jj,inum,jnum,itype,jtype; double xtmp,ytmp,ztmp,delx,dely,delz,evdwl,fpair; double rsq,r,dr,dexp,factor_lj,r2inv,r6inv,ddexp,invexp; int *ilist,*jlist,*numneigh,**firstneigh; evdwl = 0.0; if (eflag || vflag) ev_setup(eflag,vflag); else evflag = vflag_fdotr = 0; double **x = atom->x; double **f = atom->f; int *type = atom->type; int nlocal = atom->nlocal; double *special_lj = force->special_lj; int newton_pair = force->newton_pair; inum = list->inum; ilist = list->ilist; numneigh = list->numneigh; firstneigh = list->firstneigh; // loop over neighbors of my atoms for (ii = 0; ii < inum; ii++) { i = ilist[ii]; xtmp = x[i][0]; ytmp = x[i][1]; ztmp = x[i][2]; itype = type[i]; jlist = firstneigh[i]; jnum = numneigh[i]; for (jj = 0; jj < jnum; jj++) { j = jlist[jj]; factor_lj = special_lj[sbmask(j)]; j &= NEIGHMASK; delx = xtmp - x[j][0]; dely = ytmp - x[j][1]; delz = ztmp - x[j][2]; rsq = delx*delx + dely*dely + delz*delz; jtype = type[j]; if (rsq < cutsq[itype][jtype]) { r2inv = 1.0/rsq; r6inv = r2inv*r2inv*r2inv; r = sqrt(rsq); dr = r - r0[itype][jtype]; dexp = exp(-alpha[itype][jtype] * dr); ddexp = exp(-dscale * (r/rr[itype][jtype] - 1.0)); invexp = 1.0/(1+ddexp); fpair = morse1[itype][jtype] * (dexp*dexp - dexp) / r; fpair -= sscale*c[itype][jtype] * (invexp*invexp*ddexp*(-dscale/rr[itype][jtype])*r6inv) / r; fpair -= sscale*c[itype][jtype] * (6.0 * invexp * r6inv * r2inv); fpair *= factor_lj; f[i][0] += delx*fpair; f[i][1] += dely*fpair; f[i][2] += delz*fpair; if (newton_pair || j < nlocal) { f[j][0] -= delx*fpair; f[j][1] -= dely*fpair; f[j][2] -= delz*fpair; } if (eflag) { evdwl = d0[itype][jtype] * (dexp*dexp - 2.0*dexp) - sscale*c[itype][jtype]*r6inv*invexp - offset[itype][jtype]; evdwl *= factor_lj; } if (evflag) ev_tally(i,j,nlocal,newton_pair, evdwl,0.0,fpair,delx,dely,delz); } } } if (vflag_fdotr) virial_fdotr_compute(); } /* ---------------------------------------------------------------------- allocate all arrays ------------------------------------------------------------------------- */ void PairMomb::allocate() { allocated = 1; int n = atom->ntypes; memory->create(setflag,n+1,n+1,"pair:setflag"); for (int i = 1; i <= n; i++) for (int j = i; j <= n; j++) setflag[i][j] = 0; memory->create(cutsq,n+1,n+1,"pair:cutsq"); memory->create(cut,n+1,n+1,"pair:cut"); memory->create(d0,n+1,n+1,"pair:d0"); memory->create(alpha,n+1,n+1,"pair:alpha"); memory->create(r0,n+1,n+1,"pair:r0"); memory->create(c,n+1,n+1,"pair:c"); memory->create(rr,n+1,n+1,"pair:rr"); memory->create(morse1,n+1,n+1,"pair:morse1"); memory->create(offset,n+1,n+1,"pair:offset"); } /* ---------------------------------------------------------------------- global settings ------------------------------------------------------------------------- */ void PairMomb::settings(int narg, char **arg) { if (narg != 3) error->all(FLERR,"Illegal pair_style command"); cut_global = force->numeric(FLERR,arg[0]); sscale = force->numeric(FLERR,arg[1]); dscale = force->numeric(FLERR,arg[2]); // reset cutoffs that have been explicitly set if (allocated) { int i,j; for (i = 1; i <= atom->ntypes; i++) for (j = i; j <= atom->ntypes; j++) if (setflag[i][j]) cut[i][j] = cut_global; } } /* ---------------------------------------------------------------------- set coeffs for one or more type pairs ------------------------------------------------------------------------- */ void PairMomb::coeff(int narg, char **arg) { if (narg < 7 || narg > 8) error->all(FLERR,"Incorrect args for pair coefficients"); if (!allocated) allocate(); int ilo,ihi,jlo,jhi; force->bounds(FLERR,arg[0],atom->ntypes,ilo,ihi); force->bounds(FLERR,arg[1],atom->ntypes,jlo,jhi); double d0_one = force->numeric(FLERR,arg[2]); double alpha_one = force->numeric(FLERR,arg[3]); double r0_one = force->numeric(FLERR,arg[4]); double c_one = force->numeric(FLERR,arg[5]); double rr_one = force->numeric(FLERR,arg[6]); double cut_one = cut_global; if (narg == 8) cut_one = force->numeric(FLERR,arg[7]); int count = 0; for (int i = ilo; i <= ihi; i++) { for (int j = MAX(jlo,i); j <= jhi; j++) { d0[i][j] = d0_one; alpha[i][j] = alpha_one; r0[i][j] = r0_one; cut[i][j] = cut_one; c[i][j] = c_one; rr[i][j] = rr_one; setflag[i][j] = 1; count++; } } if (count == 0) error->all(FLERR,"Incorrect args for pair coefficients"); } /* ---------------------------------------------------------------------- init for one type pair i,j and corresponding j,i ------------------------------------------------------------------------- */ double PairMomb::init_one(int i, int j) { if (setflag[i][j] == 0) error->all(FLERR,"All pair coeffs are not set"); morse1[i][j] = 2.0*d0[i][j]*alpha[i][j]; if (offset_flag) { double alpha_dr = -alpha[i][j] * (cut[i][j] - r0[i][j]); offset[i][j] = d0[i][j] * (exp(2.0*alpha_dr) - 2.0*exp(alpha_dr)); } else offset[i][j] = 0.0; d0[j][i] = d0[i][j]; alpha[j][i] = alpha[i][j]; r0[j][i] = r0[i][j]; c[j][i] = c[i][j]; rr[j][i] = rr[i][j]; morse1[j][i] = morse1[i][j]; offset[j][i] = offset[i][j]; return cut[i][j]; } /* ---------------------------------------------------------------------- proc 0 writes to restart file ------------------------------------------------------------------------- */ void PairMomb::write_restart(FILE *fp) { write_restart_settings(fp); int i,j; for (i = 1; i <= atom->ntypes; i++) for (j = i; j <= atom->ntypes; j++) { fwrite(&setflag[i][j],sizeof(int),1,fp); if (setflag[i][j]) { fwrite(&d0[i][j],sizeof(double),1,fp); fwrite(&alpha[i][j],sizeof(double),1,fp); fwrite(&r0[i][j],sizeof(double),1,fp); fwrite(&c[i][j],sizeof(double),1,fp); fwrite(&rr[i][j],sizeof(double),1,fp); fwrite(&cut[i][j],sizeof(double),1,fp); } } } /* ---------------------------------------------------------------------- proc 0 reads from restart file, bcasts ------------------------------------------------------------------------- */ void PairMomb::read_restart(FILE *fp) { read_restart_settings(fp); allocate(); int i,j; int me = comm->me; for (i = 1; i <= atom->ntypes; i++) for (j = i; j <= atom->ntypes; j++) { if (me == 0) fread(&setflag[i][j],sizeof(int),1,fp); MPI_Bcast(&setflag[i][j],1,MPI_INT,0,world); if (setflag[i][j]) { if (me == 0) { fread(&d0[i][j],sizeof(double),1,fp); fread(&alpha[i][j],sizeof(double),1,fp); fread(&r0[i][j],sizeof(double),1,fp); fread(&c[i][j],sizeof(double),1,fp); fread(&rr[i][j],sizeof(double),1,fp); fread(&cut[i][j],sizeof(double),1,fp); } MPI_Bcast(&d0[i][j],1,MPI_DOUBLE,0,world); MPI_Bcast(&alpha[i][j],1,MPI_DOUBLE,0,world); MPI_Bcast(&r0[i][j],1,MPI_DOUBLE,0,world); MPI_Bcast(&c[i][j],1,MPI_DOUBLE,0,world); MPI_Bcast(&rr[i][j],1,MPI_DOUBLE,0,world); MPI_Bcast(&cut[i][j],1,MPI_DOUBLE,0,world); } } } /* ---------------------------------------------------------------------- proc 0 writes to restart file ------------------------------------------------------------------------- */ void PairMomb::write_restart_settings(FILE *fp) { fwrite(&cut_global,sizeof(double),1,fp); fwrite(&sscale,sizeof(double),1,fp); fwrite(&dscale,sizeof(double),1,fp); fwrite(&offset_flag,sizeof(int),1,fp); fwrite(&mix_flag,sizeof(int),1,fp); } /* ---------------------------------------------------------------------- proc 0 reads from restart file, bcasts ------------------------------------------------------------------------- */ void PairMomb::read_restart_settings(FILE *fp) { if (comm->me == 0) { fread(&cut_global,sizeof(double),1,fp); fread(&sscale,sizeof(double),1,fp); fread(&dscale,sizeof(double),1,fp); fread(&offset_flag,sizeof(int),1,fp); fread(&mix_flag,sizeof(int),1,fp); } MPI_Bcast(&cut_global,1,MPI_DOUBLE,0,world); MPI_Bcast(&sscale,1,MPI_DOUBLE,0,world); MPI_Bcast(&dscale,1,MPI_DOUBLE,0,world); MPI_Bcast(&offset_flag,1,MPI_INT,0,world); MPI_Bcast(&mix_flag,1,MPI_INT,0,world); } /* ---------------------------------------------------------------------- */ double PairMomb::single(int /*i*/, int /*j*/, int itype, int jtype, double rsq, double /*factor_coul*/, double factor_lj, double &fforce) { double r,dr,dexp,phi,r2inv,r6inv,ddexp,invexp; r2inv = 1.0/rsq; r6inv = r2inv*r2inv*r2inv; r = sqrt(rsq); dr = r - r0[itype][jtype]; dexp = exp(-alpha[itype][jtype] * dr); ddexp = exp(-dscale * (r/rr[itype][jtype] - 1.0)); invexp = 1.0/(1+ddexp); fforce = factor_lj * morse1[itype][jtype] * (dexp*dexp - dexp) / r; fforce -= factor_lj * sscale* c[itype][jtype] * (invexp*invexp*ddexp*(-dscale/rr[itype][jtype])*r6inv) / r; fforce -= factor_lj * sscale* c[itype][jtype] * (6.0 * invexp * r6inv * r2inv); phi = d0[itype][jtype] * (dexp*dexp - 2.0*dexp) - sscale*c[itype][jtype]*r6inv*invexp - offset[itype][jtype]; return factor_lj*phi; }